Green Synthesis of Silver-Doped Titanium Dioxide Nanostructures for Acetaminophen Degradation Under Solar Radiation
Published
Dec 16, 2022
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María Coronell, BSc
https://orcid.org/0000-0003-2760-5088
Gina Toscano-Lucas, BSc
https://orcid.org/0000-0001-9332-6824
Ricardo Solano, MSc
https://orcid.org/0000-0002-4528-2983
Adriana Herrera, PhD
https://orcid.org/0000-0002-4355-3401
https://orcid.org/0000-0003-2760-5088
Gina Toscano-Lucas, BSc
https://orcid.org/0000-0001-9332-6824
Ricardo Solano, MSc
https://orcid.org/0000-0002-4528-2983
Adriana Herrera, PhD
https://orcid.org/0000-0002-4355-3401
##plugins.themes.bootstrap3.article.details##
Abstract
Objective: In this paper, the photocatalytic degradation of acetaminophen was evaluated using silver-doped titanium dioxide nanoparticles in a cylindrical-parabolic composed photoreactor. Materials and methods: Titanium dioxide was synthesized via green synthesis using Cymbopogon citratus leaf extract and doped by silver photodeposition. Results and discussion: Morphological information shows that large agglomerates of approximately 49 nm can be attributed to the strong interaction between nanoparticles and their polycrystalline nature. The photodeposition of metallic silver reduces the surface effects, allowing a decrease in the electrostatic interaction and diameter size of the titanium dioxide, as well as the optical properties due to surface poising during the reduction of silver ions to metallic silver. The photocatalytic activity was performed to degrade acetaminophen as the drug model under visible-light radiation. The results are promising, with superior photodegradation of acetaminophen of approximately 37% and 11% for unmodified titanium dioxide and silver-doped titanium dioxide (0.75 at%) nanostructures compared to the commercial photocatalyst, respectively. Conclusions: Accordingly, the potential photocatalytic application of silver-doped titanium dioxide nanostructures is highlighted and represents a promising alternative for the photodegradation of organic compounds from wastewater eluents.
Keywords
Sustainable chemistry, surface modification, doping, photocatalysis, pharmaceuticalQuímica sostenible, modificación superficial, dopaje, fotocatálisis, fármacos
References
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[20] R. Solano, A. Herrera, D. Maestre, and A. Cremades, “Fe-TiO2 Nanoparticles Synthesized by Green Chemistry for Potential Application in Waste Water Photocatalytic Treatment,” J. Nanotechnol., vol. 2019, pp. 1–11, 2019, doi: https://doi.org/10.1155/2019/4571848
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[22] M. Pazoki, M. Parsa, and R. Farhadpour, “Removal of the hormones dexamethasone (DXM) by Ag doped on TiO2 photocatalysis,” J. Environ. Chem. Eng., vol. 4, no. 4, pp. 4426–4434, 2016, doi: https://doi.org/10.1016/j.jece.2016.09.034
[23] M. Malakootian, M. Pourshaban-Mazandarani, H. Hossaini, and M. H. Ehrampoush, “Preparation and characterization of TiO2 incorporated 13X molecular sieves for photocatalytic removal of acetaminophen from aqueous solutions,” Process Saf. Environ. Prot., vol. 104, pp. 334–345, 2016, doi: https://doi.org/10.1016/j.psep.2016.09.018
[24] J. J. Alvear-daza, J. Sanabria, J. A. Rengifo, and H. M. Gutierrez-zapata, “Simultaneous abatement of organics (2,4-dichlorophenoxyacetic acid) and inactivation of resistant wild and laboratory bacteria strains by photo-induced processes in natural groundwater samples,” Sol. Energy, vol. 171, pp. 761–768, 2018, doi: https://doi.org/10.1016/j.solener.2018.07.026
[25] R. Arumugam et al., “Scalable novel PVDF based nanocomposite foam for direct blood contact and cardiac patch applications,” J. Mech. Behav. Biomed. Mater., vol. 88, no. June, pp. 270–280, 2018, doi: https://doi.org/10.1016/j.jmbbm.2018.08.020
[26] T. M. S. Dawoud, V. Pavitra, P. Ahmad, A. Syed, and G. Nagaraju, “Photocatalytic degradation of an organic dye using Ag doped ZrO2 nanoparticles: Milk powder facilitated eco-friendly synthesis,” J. King Saud Univ. - Sci., vol. 32, no. 3, pp. 1872–1878, 2020, doi: https://doi.org/10.1016/j.jksus.2020.01.040
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How to Cite
Coronell , M., Toscano-Lucas, G., Solano, R., & Herrera, A. (2022). Green Synthesis of Silver-Doped Titanium Dioxide Nanostructures for Acetaminophen Degradation Under Solar Radiation. Ingenieria Y Universidad, 26. https://doi.org/10.11144/Javeriana.iued26.gsst
Section
Bioengineering and chemical engineering
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